The First Magic Angle Beyond the Chiral Limit in Twisted Bilayer Graphene

arXiv:2609.08347 · cond-mat.mes-hall, cond-mat.mtrl-sci · Submitted 2026-09-08 · Read on arXiv

cond-mat.mes-hall, cond-mat.mtrl-sci

Submitted: 2026-09-08

Updated: 2026-10-12

Comments: 21 pages and 13 figures

License: http://creativecommons.org/licenses/by/4.0/

The gist: We develop a squared-Hamiltonian description of twisted bilayer graphene beyond the chiral limit to explain why the first magic angle remains robust under lattice relaxation, while higher-order magic

Abstract

We develop a squared-Hamiltonian description of twisted bilayer graphene beyond the chiral limit to explain why the first magic angle remains robust under lattice relaxation, while higher-order magic angles are strongly destabilized. Starting from the non-chiral Bistritzer--MacDonald model with finite same-sublattice tunneling, we show that lattice relaxation reshapes the effective confinement landscape rather than acting as a simple perturbation of the chiral theory. A central result is that the realistic relaxation-renormalized tunneling ratio lies close to a special confinement point where the oscillatory part of the symmetric confinement potential nearly cancels. This places realistic twisted bilayer graphene near a nearly uniform confinement regime. At the same time, finite same-sublattice tunneling activates an additional inter-sublattice current-like channel that competes with the chiral orbital channel. The first magic angle survives because these confinement and current-like contributions remain balanced, whereas higher-order magic angles lose this balance through stronger remote-band hybridization and enhanced real-space localization around AA regions. Our results provide a single-particle mechanism for the breakdown of the chiral magic-angle hierarchy and clarify why the experimentally relevant first magic angle remains the most stable remnant of the chiral flat-band structure.

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